[ RadSafe ] measurement of Kr-85 using Overhoff 400 portable tritium monitor
JGinniver at aol.com
JGinniver at aol.com
Tue Jul 25 17:13:42 CDT 2006
Has anyone on radsafe any experience of calculating Kr-85 concentrations
from measurements using a gas flow ion chamber?
It would appear that one of the facilities at the site where I work may have
discharged some Kr-85. At the time that the discharge is thought to have
occured several measurements were made using a portable tritium monitor
(Overhoff Model 400), these indicated measurable amounts of tritium in the stack
discharge from a series of shielded caves containing spent nuclear fuel.
Subsequent analysis of the tritium bubblers on the vent line indicate that no
tritium was present. As a result it is believed that a discharge of radioactive
gas has occurred, and because of the nature of the facility this is likely to
have been Kr-85.
While the discharge was within allowable limits, the operators of the
facility would like a better estimate of the activity discharged and the only
available measurements are from the portable tritium monitors.
Having refreshed my memory with my copy of Knoll, it is clear that this is
not easy to do as the majority of the energy from the beta emissions is likely
to have been deposited outside of the detection chambers in the instrument.
The only reference given in Knoll for further guidance is T. Torii, Nucl.
Instrumen. Meth. A356, 255 (1995) a search on google has turned up the
following,
T. Torii: Ionization efficiency of a gas-flow ion chamber used for
measuring radioactive gases by Monte Carlo simulation
Nucl. Instr. Methods A356(1955)255-263.
which I'm assuming is the one mentioned in Knoll? Does anyone have an
electronic copy I could have to look at, or does anyone have experience of trying
to do similar calculations?
Regards,
Julian
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