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Regarding Pu-238, and SNAP 9-A
In a recent thread, a discussion, or reference was made, regarding the
reentry of a SNAP reactor and the subsequent Pu-238 release and
dispersion across the stratosphere. Merrill Eisenbud, in his book,
"Environmental Radioactivity ..." discusses the abortive reentry of
the SNAP 9-A satellite April 21, 1964. This satellite failed to reach
orbital velocity and reentered the atmosphere at 150,000 ft. over the
Indian Ocean. The power unit contained about 17,000 Ci of Pu-238.
The Pu was first detected at 108,000 feet four months following the
abort. The stratospheric distribution of the debris during the next
several years followed the predictions that had been made on the basis
of transport models of ths stratosphere developed through studies of
the behavior of debris from weapons testing, however, the
concentrations of Pu-238 was lower in ground level air than had been
predicted. About 95% of the Pu originally injected had been deposited
by the end of 1970. Particle size analysis indicated that the
particle size ranged from 5 to 58 um. The Pu content of ground level
air as monitored by de Bartoli and Gaglione (1969) et al, concludes
the 50 year commitment to the pulmonary lymph node from Pu exposure
between 1961 and 1968 was 36 mRem. - source Eisenbud, p. 365-366,
"Environmental Radioactivity.