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H-3 - another theory
Let me throw another possibility out:
Electrons, contrary to what is commonly believed, or at least what is
convenient to assume, DO NOT have a finite range. Other processes other than
the CSDA range are involved - straggling, etc. See Turner or any of Berger's
work. The upshot is that you can have some penetration of electrons at depths
>> CSDA range. Think of it like a tunnelling effect. For example, see Table 9
of MIRD 5; the x90 for a 20 kev
electron is 6E-4 cm in water. Now, a 1 mg/cm^2 wall is about 10E-4 cm, assuming
unit density. So, if you have a large enough activity source, even with few
particles at or near Emax, and a container and detector with walls > range,
I'll bet you're detecting some H-3 beta particles.
I've seen this phenomena with P-32; don't try shielding 100 mCi with 1 cm
lucite - you'll need more.
Lynn McGuire
Univ. of Ark. Med. Sciences