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Re: Naturally occurring Pu-244
Phil,
This may not be much help, but maybe $0.01 worth:
Holleman JW, PA Quiggins, BD Chilton, MS Uziel, HA Pfuderer, and JA Longmire. March 1987. Worldwide Fallout of Plutonium from Nuclear Weapons Tests. Rep. ORNL-6315. Oak Ridge National Laboratory.
This report focuses on fallout and deposition of Pu-238 and Pu-239,240. It does have a very brief discussion of the composition of fallout, which does NOT specifically mention Pu-244. It does indicate that "...No transuranics above 246Cm were identified in reactor material. However, transuranics from 242Pu to 255Es have been identified in bomb debris at levels of 10-3 to 10-8 [i.e., E-3 to E-8] relative to 239Pu as 1."
This would seem to say that there could be some Pu-244 from weapons testing fallout, but that the levels would be quite small. And smaller now with a few half-lives of decay.
Good luck.
Duane.
Duane Schmidt
U.S. Nuclear Regulatory Commission
Office of Nuclear Material Safety and Safeguards
Division of Waste Management
Decommissioning Branch
dws2@nrc.gov
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Date: Wed, 04 Sep 2002 16:59:44 -0600
From: "Philip Egidi" <phil.egidi@state.co.us>
Subject: Naturally occurring Pu-244
RADSTERS,
I have a time critical response to put out to a member of the public
about naturally occurring Pu-244.
I have looked at NCRP 94, Kocher, UNSCEAR, Eisenbud/Gessell, Schlien,
and the prestigious Google. I don't have a whole lot to show for it
yet.
Does anyone have (preferable electronic) any papers or references on
the occurrence and properties of naturally occurring Pu-244?
Thanks,
Phil Egidi
phil.egidi@state.co.us
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